Diffraction, Fourier Optics and Imaging in .NET

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must align themselves to obtain the desired additive effect. Also, it is helpful if the molecules are transparent at the laser wavelength. The second-order effect can be used to obtain frequency doubling through second harmonic frequency mixing, light-modulation through a linear electro-optical effect, and intensity enhancement through optical recti cation. It has been suggested (98) that the one-dimensional coordination polymer KTiO(PO4 ) (also known as KTP) has a high NLO coef cient, a high optical damage threshold, a low threshold power, and a low phase-matching sensitivity that should make it better than the two materials currently used, KH2 PO4 and LiNbO3 KTiO PO4 consists of a zigzag TiDO TiDO chain with unequal bond lengths (<1.75 vs. >2.10 A) to give the noncentrosymmetric structure required for second-order NLO. Phosphate groups complete a crosslinked distorted octahedral structure about each titanium(IV) ion in the ( TiDO)n chain. Other one-dimensional metal coordination polymers have been investigated as well. For example, [(salen)MIII - -O3 SCH2 NHC5 H5 N]n , where M D Cr, Mn, Fe, Co, shows small amounts of second-order NLO properties, but the adjacent salen rings in each chain are almost perpendicular to each other, which causes a diminished ef ciency. The third-order ( ) term is responsible for the generation of new frequencies using third harmonics. The nature of the best types of molecules is still not totally settled; however, linear or rigid-rod metal-containing polymers show considerable promise (96). Other solid-state polymeric coordination compounds are also quite promising (98, 99) as well as composites consisting of inorganic oxides and conjugated polymers (97) and selected phthalocyaninato metal species (83). This is an area in which inorganic polymers may become increasingly important.
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Figure 8.3 Structure of salicylic acid (cf. DQ 8.1).
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The list step of this refactoring is to compile, deploy, and test the changes. Now that this refactoring is in place, co-located invocations between Session fa ades and colocated Entity Beans should perform much better. Finally, this refactoring has operated under the assumption of switching a bean from remote to local interfaces. However, it is possible for a bean to support both types of interfaces simultaneously. To accomplish this, simply be additive in applying this refactoring. For example, instead of modifying the AccountHome.java and Account .java files, add two new ones AccountLocalHome.java and AccountLocal.java that contain the local interface definitions. Likewise, instead of replacing the remote tags within the Account s deployment descriptor, simply add the local tags. This way, clients can choose either to continue using the Account bean via its remote interface, or to use the new local interface. This approach can be used to incrementally introduce local interfaces to an application.
feature provides a lower interaction between the side groups than the trans, trans structure observed for most of the siloxanes. Whereas Si O and P N pairs are isoelectronic (each supply 10 valence electrons), traditionally the phosphazenes are considered as unsaturated compounds with one pair of the electrons per repeating unit relegated to P d N p bonding and the other non-sigma bonding pair as a lone pair on the nitrogen. Although this provides alternating single and double bonds, the bond lengths are equal in the ring systems that are analogous to the polymer chains, so delocalization seems logical as shown in Figure 1.25. However, no matter how large the phosphazene ring or chain, no shifts in electronic transistions are observed. This leads to the speculation that the d-orbital nodes stop the delocalization at each phosphorus atom. On the other hand, siloxanes are considered saturated compounds with the opening of the Si O Si bond angle by Si d O p bonding, with the electrons being from the so-called oxygen lone-pairs. If all four valence electrons not involved in sigma bonding in the phosphazenes were placed as lone pairs on the nitrogen atoms in an analogous fashion, each nitrogen would have an electron excess (a negative charge) and each phosphorus would have an electron shortage (a positive charge). Substituents on polyphosphazenes are not limited to organic groups. Derivatives with iron and ruthenium bonded directly to the phosphorus atoms are known (Fig. 1.26a) and cyclopentadienyl groups on the phosphorus atoms have been used to prepare anchored ferrocene derivatives (Fig. 1.26b,c), too. Note that both cyclopentadienyl (Cp) entities are on the phosphorus atoms in the latter case. The PNPCpFeCp ring strain in the trimer that is used to prepare the polymer allows low-temperature ring-opening polymerization as noted in 2. Attempts to bind metal ions on the lone pairs of the nitrogen atoms have not been overly successful. However, a derivative related to cisplatin, cis-diamminedichloroplatinum(II) (Fig. 1.26d), has been prepared with a maximum loading of about 1 platinum center per 17 phosphazene units. Polyheterophosphazenes (16) are closely related to the polyphosphazenes. They include the polycarbophosphazenes, the polythiophosphazenes, and the
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